Ordering Phenomena in Rare-Earth Nickelate Heterostructures

Ordering Phenomena in Rare-Earth Nickelate Heterostructures
Author :
Publisher : Springer
Total Pages : 159
Release :
ISBN-10 : 9783319605319
ISBN-13 : 3319605313
Rating : 4/5 (313 Downloads)

Book Synopsis Ordering Phenomena in Rare-Earth Nickelate Heterostructures by : Matthias Hepting

Download or read book Ordering Phenomena in Rare-Earth Nickelate Heterostructures written by Matthias Hepting and published by Springer. This book was released on 2017-06-28 with total page 159 pages. Available in PDF, EPUB and Kindle. Book excerpt: This thesis presents an experimental study of ordering phenomena in rare-earth nickelate-based heterostructures by means of inelastic Raman light scattering and elastic resonant x-ray scattering (RXS). Further, it demonstrates that the amplitude ratio of magnetic moments at neighboring nickel sites can be accurately determined by RXS in combination with a correlated double cluster model, and controlled experimentally through structural pinning of the oxygen positions in the crystal lattice. The two key outcomes of the thesis are: (a) demonstrating full control over the charge/bond and spin order parameters in specifically designed praseodymium nickelate heterostructures and observation of a novel spin density wave phase in absence of the charge/bond order parameter, which confirms theoretical predictions of a spin density wave phase driven by spatial confinement of the conduction electrons; and (b) assessing the thickness-induced crossover between collinear and non-collinear spin structures in neodymium nickelate slabs, which is correctly predicted by drawing on density functional theory.


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